High Resolution Simulations of Pollution Vertical Stratification over Santiago and its Transport to the Chilean Andes

Abstract:

Santiago, Chile (33.5 S, 70.5 W, 500 m.a.s.l., population 7 millions) is a large city situated in a basin surrounded by the Andes in the East and smaller mountain ranges to the North, West, and South. It is plagued by abnormally high pollution levels for its size due to climatological and topological features. To date, it is unclear how far the urban pollution plume reaches up the mountain. Here we explore the region’s complex atmospheric circulation and particularly the transport of black carbon (BC) using a state of the art numerical model (WRF-Chem, Weather Research and Forecasting model).

Observations indicate the presence of multiple layers within the boundary layer, as well as the occurrence of uncoupled layers above the boundary layer. Here we explore mechanisms within our simulation that may explain these features. Our results suggest that they may correspond to residual layers that are produced by recirculation along mountain slopes due to the complex terrain around the city.

In late August 2013, a short multi-platform measuring campaign (DIVERSOL) took place in the Santiago basin, providing the first vertical profiles of BC, accompanied by meteorological soundings. We analyze the dispersion of a quasi-passive tracer (carbon monoxide) of black carbon in our simulation to improve our understanding of the governing mixing and transport processes. We also perform sensitivity studies with respect to vertical resolution and turbulence schemes, contrasting our results against DIVERSOL data. Our simulations suggest that pollutants emitted in Santiago could reach the high regions of Andes mountains during the afternoon circulation, thus affecting local glaciers.

With an entire year of simulation we find that the stratification of pollutants within the basin displays a seasonal signal, as well as a capacity to reach the Chilean Andes and affect the Andean cryosphere.