The Role of African Dust Particles on Cloud Chemistry and Microphysics in a Tropical Montane Cloud Forest in the Caribbean

Abstract:

Huge amounts of African dust travels thousands of kilometers from the Sahara and Sahel regions to the Caribbean, northern South America and southern North America. However, not much is understood about how the aging process that takes place during transport changes dust properties, and how it affects cloud’s composition and microphysics. In order to improve our understanding of the role of long-range transported African dust (LRTAD) in cloud formation processes we had field campaigns measuring dust physical and chemical properties in summers of 2013, 2014 and 2015, as part of the Puerto Rico African Dust and Cloud Study (PRADACS), and of the Luquillo Critical Zone Observatory (LCZO). Measurements were performed at the tropical montane cloud forest (TMCF) of Pico del Este (PE, 1051 masl) and at the nature reserve of Cabezas de San Juan (CSJ, 60 masl). In both ground stations we monitored meteorological parameters (e.g., temperature, wind speed, wind direction). At CSJ, we measured light absorption and scattering at three wavelengths (467, 528 and 652 nm). At PE we collected cloud and rainwater for chemical analyses and monitored cloud microphysical properties (e.g., liquid water content, droplet size distribution, droplet number concentration, effective diameter and median volume diameter). Summer 2015 was the first attempt to characterize microphysical properties of the summer period (June to August) at PE, where dust is in its higher concentrations of the year. Samples were classified using data from models and satellites together with CSJ measurements as low or high dust influenced. Soluble ions, insoluble trace metals, pH, conductivity, total and dissolved organic carbon and total and dissolved nitrogen were measured for cloud and rainwater. Enrichment factor analysis was used to determine sea and crustal contribution of species by sample, as well as the neutralization factor and fractional acidity. Some preliminary results show cloud water conductivity for low and high dust periods was 47.7 vs 81.1 mS/cm, respectively, and for rainwater was 12.8 mS/cm vs 15.0 mS/cm. pH showed differences no larger than 11% for both 2013 and 2014 periods. Also, microphysical data from summer 2013 suggest that dust may be hindering cloud formation processes. Detailed results from all campaigns will be presented at the meeting.